Enhanced photocatalysis using metal-organic framework MIL-101(Fe) for crude oil degradation in oil-polluted water

LIANG Yuning; WANG Baohui; LI Shuohui; CHI Weimeng; BI Mingchun; LIU Yuxuan; WANG Yiran; YAO Ming; ZHANG Tianying; CHEN Ying

doi:10.1016/S1872-5813(23)60396-2

Volume 52 Issue 4

Apr. 2024

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Article Navigation > Journal of Fuel Chemistry and Technology > 2024 > 52(4): 607-618

LIANG Yuning, WANG Baohui, LI Shuohui, CHI Weimeng, BI Mingchun, LIU Yuxuan, WANG Yiran, YAO Ming, ZHANG Tianying, CHEN Ying. Enhanced photocatalysis using metal-organic framework MIL-101(Fe) for crude oil degradation in oil-polluted water[J]. Journal of Fuel Chemistry and Technology, 2024, 52(4): 607-618. doi: 10.1016/S1872-5813(23)60396-2

Citation:

LIANG Yuning, WANG Baohui, LI Shuohui, CHI Weimeng, BI Mingchun, LIU Yuxuan, WANG Yiran, YAO Ming, ZHANG Tianying, CHEN Ying. Enhanced photocatalysis using metal-organic framework MIL-101(Fe) for crude oil degradation in oil-polluted water[J]. Journal of Fuel Chemistry and Technology, 2024, 52(4): 607-618. doi: 10.1016/S1872-5813(23)60396-2

Citation:

LIANG Yuning, WANG Baohui, LI Shuohui, CHI Weimeng, BI Mingchun, LIU Yuxuan, WANG Yiran, YAO Ming, ZHANG Tianying, CHEN Ying. Enhanced photocatalysis using metal-organic framework MIL-101(Fe) for crude oil degradation in oil-polluted water[J]. Journal of Fuel Chemistry and Technology, 2024, 52(4): 607-618. doi: 10.1016/S1872-5813(23)60396-2

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Enhanced photocatalysis using metal-organic framework MIL-101(Fe) for crude oil degradation in oil-polluted water

doi: 10.1016/S1872-5813(23)60396-2

LIANG Yuning^1
,,
WANG Baohui^{1
,
,},
LI Shuohui^1
,,
CHI Weimeng¹,
BI Mingchun^1
,,
LIU Yuxuan^1
,,
WANG Yiran^1
,,
YAO Ming^1
,,
ZHANG Tianying^2
,,
CHEN Ying^{1
,
,}

1.
Key Laboratory of Oil and Natural Gas Processing, School of Chemistry and Chemical Engineering, Northeast Petroleum University, Daqing 163318, China
2.
Operation Team of Daqing Oil Field Production Testing Branch, Daqing 163318, China

More Information

Corresponding author: Tel: 18345996681, E-mail: wangbh@nepu.edu.cn; Tel:18345996681, E-mail:chenying648617@163.com chenying648617@163.com
Received Date: 2023-07-04
Accepted Date: 2023-10-18
Rev Recd Date: 2023-10-12

Available Online: 2023-11-10

Publish Date: 2024-04-03

Abstract

Abstract

A stable metal-organic framework (MOF), MIL-101(Fe), was successfully synthesised using a solvothermal method and employed as a novel photocatalyst for degrading crude oil in oilfield wastewater. Through optimisation of reaction conditions, the following optimal parameters were determined: a dark reaction time of 30 min, a light reaction time of 30 min, a pH of 5.5, a catalyst amount of 150 mg/L, and a reaction temperature of 303.15 K. Under these reaction conditions, an impressive removal of 94.73% was achieved. This study represents the first application of Fe-based MOFs in the photocatalytic degradation of oilfield wastewater. MIL-101(Fe) notably demonstrated excellent stability under mild acid conditions and can be efficiently recycled. These findings offer valuable insights into using MIL-101(Fe) as a promising material for industrial applications in removing crude oil from oil-polluted water through photocatalytic degradation.
- MIL-101(Fe),
- MOF,
- photocatalysis,
- solvothermal,
- oilfield wastewater,
- degradation

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References(35)

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